银纳米团簇颗粒局域表面等离激元增强荧光

doi:10.3969/j.issn.0255-8297.2016.02.007

应用科学学报 ›› 2016, Vol. 34 ›› Issue (2): 171-176.doi: 10.3969/j.issn.0255-8297.2016.02.007

银纳米团簇颗粒局域表面等离激元增强荧光

张涛¹, 徐荣青^1,2, 谌静², 邓贝³

1. 南京邮电大学光电工程学院, 南京 210023;
2. 南京邮电大学电子科学与工程学院, 南京 210023;
3. 香港城市大学物理与材料科学系, 香港 999077

收稿日期:2013-10-07 修回日期:2013-12-17 出版日期:2016-03-30 发布日期:2016-03-30
通信作者: 谌静,博士,副教授,研究方向:表面等离激元和亚波长光学、表面增强荧光及表面增强拉曼散射,E-mail:jchen@njupt.edu.cn E-mail:jchen@njupt.edu.cn
基金资助:
国家自然科学基金(No.11304159, No.60778007);教育部博士点基金(No.20133223120006);南京邮电大学引进人才科研启动基金(No.NY213023)资助

Localized Surface Plasmon Enhanced Fluorescence on Silver Nanoclusters

ZHANG Tao¹, XU Rong-qing^1,2, CHEN Jing², DENG Bei³

1. School of Optoelectronic Engineering, Nanjing University of Posts and Telecommunications, Nanjing 210023, China;
2. College of Electronic Science and Engineering, Nanjing University of Posts and Telecommunications, Nanjing 210023, China;
3. Department of Physics and Materials Science, City University of Hong Kong, Hong Kong, 999077, China

Received:2013-10-07 Revised:2013-12-17 Online:2016-03-30 Published:2016-03-30

摘要/Abstract

摘要： 采用基于磁控等离子体团簇束流源的低能团簇束流沉积在石英衬底上制备了银纳米团簇颗粒,并测量了其透射光谱.将二氧化硅荧光纳米球分别分散在裸石英片和有银纳米团簇颗粒的石英片上,用波长为410 nm的激光激发,结果表明有银钠米团簇颗粒的荧光发射强度与没有银纳米团簇颗粒的荧光发射强度相比,增强倍数达5.3倍.最后,用Mie散射理论数值计算单个银纳米球颗粒在其表面等离激元共振位置处的电场强度分布,据此对实验结果进行了合理的解释.

关键词: 银纳米团簇颗粒, 表面等离激元, 表面增强荧光, Mie散射理论

Abstract: Using low energy cluster beam deposition based on magnetron plasma gas aggregation cluster source, we fabricated silver nanoclusters on a quartz substrate and measured its transmittance spectrum. Then we dispersed SiO₂ fluorescent nanospheres separately on bare quartz substrates and quartz substrates with silver nanoclusters. We found that the fluorescence intensity with silver nanoclusters was 5.3 larger than that without silver nanoclusters. Finally, we used the Mie scattering theory to numerically calculate the electric field intensity distributions of a single silver nanosphere where surface plasmon resonance existed. We give a reasonable explanation for the experimental results.

Key words: silver nanocluster, surface plasmon, surface enhanced fluorescence, Mie scattering theory

中图分类号:

O657.32

张涛, 徐荣青, 谌静, 邓贝. 银纳米团簇颗粒局域表面等离激元增强荧光[J]. 应用科学学报, 2016, 34(2): 171-176.

ZHANG Tao, XU Rong-qing, CHEN Jing, DENG Bei. Localized Surface Plasmon Enhanced Fluorescence on Silver Nanoclusters[J]. Journal of Applied Sciences, 2016, 34(2): 171-176.

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银纳米团簇颗粒局域表面等离激元增强荧光

Localized Surface Plasmon Enhanced Fluorescence on Silver Nanoclusters

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